Mass Spectrometric Investigation of 2-Methoxyethanol and 2-Ethoxyethanol Clusters: Magic Numbers and Structural Implications

Abstract

In this paper we present the results of our mass spectrometric investigations for van der Waals clusters of 2-methoxyethanol and 2- ethoxyethanol. The cluster mass spectra were acquired for a variety of expansion conditions and electron energies. The protonated alkoxyethanol cluster ions (AE)nH(+) form the dominant cluster ion series. A number of fragment ions, that may arise from an unprotonated and/or a protonated alkoxyethanol molecular ion, were solvated by additional alkoxyethanol molecules. The (AE)n(H20)mH(+) ions were observed with significant intensities only for n >/= 5 in neat as well as mixed alkoxyethanol/water expansions. It was also found that (AE) n (H20)m H(+) cluster ions which satisfy the condition n = 2 (m + 2), for m = 1 and 2, have enhanced ion intensities. The various models that may explain the behavior of (AE)n(H20)mH(+) are discussed.

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Document Details

Document Type
Technical Report
Publication Date
Apr 03, 1993
Accession Number
ADA262822

Entities

People

  • Gopal Vaidyanathan
  • James F. Garvey
  • William J. Herron

Organizations

  • University at Buffalo

Tags

Communities of Interest

  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alcohols
  • Chemical Reactions
  • Chemistry
  • Dipole Moments
  • Electron Energy
  • Electrons
  • Energy
  • Hydrogen Bonds
  • Intensity
  • Mass Spectra
  • Mass Spectrometers
  • Molecules
  • New York
  • Organic Chemistry
  • Physical Chemistry
  • Spectra
  • Stagnation Pressure

Fields of Study

  • Chemistry

Readers

  • Quantum Chemistry

Technology Areas

  • Microelectronics