Femtosecond Laser Studies of Excited State Dynamics

Abstract

Considerable progress has been made in the two main (and interrelated) areas in which the recent research has been focussed. These are (a) the development of novel, intense, femtosecond-time-scale, VUV laser sources, and (b) the development of femtosecond-time-scale, transition-state absorption spectroscopy of photodissociating gas-phase molecules. In both of these areas, some trails have been blazed that will undoubtedly soon be followed by others. A third area of investigation was to examine the possibility of two- photon amplification in the molecular system diphenyl hexatriene (DPH). Here the critical experiment still remains to be done. However, researchers were able to show that DPH does satisfy one stringent requirement for a potential two-photon amplifying system, namely, that it be completely stable against one-photon lasing under conditions of very heavy optical pumping..... Femtosecond-Time- Scale, Gas phase molecules, Photons, Lasers, Diphenyl hexatriene, Optical pumping.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1993
Accession Number
ADA263708

Entities

People

  • J. H. Glownia
  • Peter P. Sorokin

Organizations

  • IBM Thomas J. Watson Research Center

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Amplification
  • Amplifiers
  • Difference Frequency
  • Femtosecond Lasers
  • Femtosecond Time
  • Frequency
  • Laser Beams
  • Laser Pulses
  • Lasers
  • Measurement
  • Molecules
  • Nanosecond Time
  • Optical Pumping
  • Spectroscopy
  • Wave Mixing

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Optical Physics and Photonics.
  • Systems Analysis and Design

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers