Polymer-Polymer Interactions

Abstract

Our approach for understanding polymer-polymer interactions is to measure heats of mixing of small molecule analogs. In particular, we have focused on small molecule analogs of polystyrene (PS) and Poly (2, 6 dimethyl phenylene oxide) (PPO). this well-known system is miscible, but the origin of its miscibility has perplexed investigators for over 25 years. Our measurements and associated molecular mechanics/Monte Carlo calculations have firmly established that the two methyl groups on PPO play a significant role in affecting miscibility. We have developed two equation of state models for hydrogen bonding interactions. They represent a significant advance in our understanding of hydrogen bonding interactions in both polymeric and non- polymeric systems. The models have been successfully applied to a variety of systems that include supercritical fluids. solubility of gases in liquid polymers has been treated theoretically using the lattice-fluid model.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 1993
Accession Number
ADA265304

Entities

People

  • Donald R. Paul
  • Isaac C. Sánchez

Organizations

  • University of Texas at Austin

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alkenes
  • Aromatic Hydrocarbons
  • Bulk Modulus
  • Chemistry
  • Chlorinated Hydrocarbons
  • Cyclic Hydrocarbons
  • Energy
  • Equations
  • Free Energy
  • Hydrocarbons
  • Mechanics
  • Molecules
  • Physical Properties
  • Polymers
  • Small Molecules
  • Solubility
  • Solvents

Fields of Study

  • Chemistry

Readers

  • Polymer Science and Technology
  • Theoretical Analysis.