Amide and Tetrazene Complexes of Transition and Main Group Elements as Precursors for the Low Temperature Synthesis of Elemental Nitrides

Abstract

Tetrazene complexes and nitrene compounds derived therefrom were prepared. Attempts to use these compounds as precursors to metal nitride species failed. Metal acetylide complexes were prepared and examined by X-ray crystallography. Electrochemical procedures to deposit aluminum nitride films were explored using nonaqueous solvents. The reaction of several organometallics with azide ion was studied. The disproportionation reactions between 17-electron chromium triad radicals and various nucleophiles were characterized by infrared spectroscopy. The formation of reversible adducts from the reaction between trivalent phosphorus donor ligands and unsaturated organic carbonyl compounds was observed.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
May 01, 1993
Accession Number
ADA266246

Entities

People

  • William C. Trogler

Organizations

  • University of California, San Diego

Tags

DTIC Thesaurus Topics

  • Aluminum Nitrides
  • Chemistry
  • Diamond Films
  • Electrons
  • Elements
  • Infrared Spectroscopy
  • Low Temperature
  • Metals
  • Nitrides
  • Nitrogen
  • Nitrogen Compounds
  • Precursors
  • Spectroscopy
  • Substitution Reactions
  • Tetrazenes
  • X Rays
  • X-Ray Crystallography

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene