Theoretical Prediction of the UV Adsorption and Fluorescence Spectra of Tyrosine and Phenylalanine

Abstract

This report presents a theoretical study of the ground state and of the first excited state of phenylalanine and tyrosine to interpret the excitation absorption and the fluorescence emission spectra of the two molecules. The computations are performed with the Gaussian 90 Program Package using 3-21G basis sets. The ground state is computed with the HF option and the excited state with the Configuration Interaction, Single (CIS) Excitations option only. This report optimized the molecular geometries of both the ground and excited states and computed the excitation energies at both geometries. In conclusion, the excited state is due to a superposition of excitations from bonding orbitals in the alanine chain to a pi orbital in the benzene ring and to an orbital in the C-C bond attached to the ring.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 1993
Accession Number
ADA266970

Entities

People

  • Hendrik F. Hameka
  • James O. Jensen

Organizations

  • Battelle Memorial Institute

Tags

Communities of Interest

  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Amino Acids
  • Aqueous Solutions
  • Aromatic Amino Acids
  • Atomic Charge
  • Charge Density
  • Computations
  • Crystal Structure
  • Emission Spectra
  • Excitation
  • First Principles Calculations
  • Frequency
  • Geometry
  • Ground State
  • Molecules
  • Spectra
  • Tryptophan

Fields of Study

  • Physics

Readers

  • Analytical Chemistry
  • Quantum Chemistry

Technology Areas

  • Space