Crystallization and Microstructural Control of Ferroelectric Thin-Films and Glass-Ceramics

Abstract

Research on solution-derived ferroelectric thin-films and melt- derived ferroelectric glass-ceramics is being conducted in parallel with considerable overlap in the compositions studied and the evaluations of the crystallization behavior, microstructural development, and resulting properties. By establishing the similarities and differences between the two systems, techniques developed for one technology can then be applied to advance the other. The investigation is focusing on the Pb(ZrxTil-x)O3-Pb5Ge3O11 (PZTPG) system. Compositions from this system combine the glass forming ability and low processing temperatures of PG with the excellent electrical properties of PZT. These compositions crystallize into multiple ferroelectric phases, and thus by controlling the ratios of these phases unique combinations of properties may be possible. The high PG compositions are being investigated for pyroelectric applications, while the high PZT compositions are of interest for piezoelectric applications. This program appears to be the first to investigate melt-derived PG-PZT compositions, crystallize multiple ferroelectric phases, and crystallize PZT from a glass. This research demonstrates the feasibility of developing piezoelectric glass-ceramics with low processing temperatures that utilize powder processing techniques, such as pressing, screen printing, or tape casting, and indicates the potential of incorporation of these materials into low-fired multilayer packages as a sensors or actuators.

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Document Details

Document Type
Technical Report
Publication Date
Sep 30, 1993
Accession Number
ADA273767

Entities

People

  • Michael J. Haun

Organizations

  • Colorado School of Mines

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Ceramic Materials
  • Chemistry
  • Composite Materials
  • Crystallization
  • Crystals
  • Curie Temperature
  • Dissipation Factor
  • Electrical Properties
  • Electronic Components
  • Heat Energy
  • Heat Treatment
  • Materials
  • Materials Engineering
  • Materials Processing
  • Materials Science
  • Phase Transformations
  • Transition Temperature

Fields of Study

  • Materials science

Readers

  • Computational Modeling and Simulation
  • Computer Science/Computer Engineering/Data Science/Digital Signal Processing.
  • Materials Science and Engineering.