Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometric Study of Singly and Doubly Charged Organometallic Complexes

Abstract

An external source electrospray ionization (ESI) Fourier transform ion cyclotron resonance (FTICR) mass spectrometer has been used to study the organometallic complexes Ag2(DPM)2(BF4)2 (where DPM = bis-diphenylphosphino- methane), Ag2(DPM)3(BF4)2 and Ru(II)(bp)3(PF6)2 (where bpy = 2,2'-bipyridyl). The high mass resolution and accurate mass assignment of parent and collisionally induced dissociation (CID) fragment ions provided structural information on these organometallic complexes. CID in the capillary/skimmer region and inside the FTICR analyzer cell were performed on these complexes and results from each type of experiment were compared. Important fragmentation pathways and reaction types, including bond cleavage, ligand loss, and ligand substitution were identified. Electrospray ionization, Organometallic complexes, Fourier transform ion cyclotron resonance mass spectrometry.

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Document Details

Document Type
Technical Report
Publication Date
May 27, 1994
Accession Number
ADA279899

Entities

People

  • C. Stacey
  • D. E. Richardson
  • G. H. Kruppa
  • J. R. Eyler
  • R. Ramanathan

Organizations

  • University of Florida

Tags

DTIC Thesaurus Topics

  • Analyzers
  • Chemical Synthesis
  • Chemistry
  • Cyclotron Resonance
  • Cyclotrons
  • Dissociation
  • Electrospray
  • Electrospray Ionization
  • Ionization
  • Mass Spectra
  • Mass Spectrometers
  • Mass Spectrometry
  • Resonance
  • Spectrometers
  • Spectrometry
  • United States
  • United States Government

Fields of Study

  • Chemistry

Readers

  • Molecular Photonics/Laser Physics
  • Quantum Chemistry