Thermal Polymerization of Styrene in the Presence of Stable Radicals and Inhibitors

Abstract

Thermal polymerization of styrene in the presence of several radical scavengers and inhibitors was investigated. Rates, molecular weights and polydispersities depend on the nature of the scavenger, on its concentration and reaction temperature. In the best controlled systems, molecular weights up to M sub n approx. 10,000 and polydispersities M sub w/M sub n approx. 1.2 were observed. It is proposed that in addition to the reversible activation by the homolytic cleavage of the 'dormant' (P-R) species, degenerative chain transfer reactions may be involved.

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Document Details

Document Type
Technical Report
Publication Date
Jun 30, 1994
Accession Number
ADA280926

Entities

People

  • Daniela Mardare
  • Krzysztof Matyjaszewski

Organizations

  • Carnegie Mellon University

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Abstracts
  • Chemical Reactions
  • Chemistry
  • Classification
  • Conversion
  • Diazo Compounds
  • Governments
  • Inhibitors
  • Military Research
  • Molecular Weight
  • Organometallic Compounds
  • Polymerization
  • Reversible
  • Styrenes
  • United States
  • United States Government

Readers

  • Organic Chemistry