Epitaxial MOCVD of Thin Film Ceramics for Pyroelectric Detectors

Abstract

The objective of this research is to increase the sensitivity of pyroelectric detectors by growing a thin-film single crystal of lead-titanate (PTO) on cobalt-silicide (CoSi2) on silicon using metalorganic chemical vapor deposition (MOCVD). A thermal isolated, aligned film should increase detectivity. In Phase I of this research Spire demonstrated MOCVD of PTO on CoSi2 on silicon by MOCVD using a diffusion barrier between the films. Small capacitors were fabricated and the dielectric constant was formed to vary with temperature as expected. Multiple films were required to preserve the heteroepitaxial crystal structure while preventing chemical interactions and interdiffusion. Formation of silicon-dioxide prevents direct deposition of epitaxial oxide films on silicon, so that CoSi2 was deposited first. This was followed by laser ablation deposition of the conducting film yttrium-barium- copper-oxide to prevent inter-diffusion of lead. The PTO film was then put down by MOCVD, and the structure was verified by X-ray diffraction.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1993
Accession Number
ADA281397

Tags

DTIC Thesaurus Topics

  • Backscattering
  • Chemical Reactions
  • Chemical Vapor Deposition
  • Crystals
  • Curie Temperature
  • Detectors
  • Dielectric Permittivity
  • Electrical Measurement
  • Epitaxial Growth
  • High Temperature
  • Integrated Circuits
  • Materials
  • Measurement
  • Piezoelectric Crystals
  • Spectroscopy
  • Thin Films
  • X-Ray Diffraction

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Powder metallurgy of Titanium alloys.
  • Semiconductor Device Technology

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition