Enzyme Catalyzed 2-D Polymerization of Phenol and Aniline Derivatives on a Langmuir-Blodgett Through

Abstract

Previous studies have shown that polymeric materials may be synthesized from substituted phenols and aromatic amine compounds through a Horseradish Peroxidase (HRP) enzyme catalyzed reaction in the bulk. We have developed a novel approach for this enzyme mediated polymer synthesis which involves in-situ polymerization using a Langmuir-Blodgett (LB) technique. Here, the LB technique is used to organize and manipulate the reactants during polymerization at the molecular level. This methodology provides direct control over the resulting structure, order and orientation of the final polymeric material. This enhanced control leads to improved processability, tensile strength, and functional properties for the polymers. This new synthetic approach and the resultant ordered polymer product can form the basis for intelligent material design. Langmuir-Blodgett, Horseradish peroxidase, Aromatic amine, Enzyme, Phenol.

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Document Details

Document Type
Technical Report
Publication Date
Dec 31, 1992
Accession Number
ADA281660

Entities

People

  • B. K. Mandal
  • D. L. Kaplan
  • F. Bruno
  • J. A. Akkara
  • L. A. Samuelson

Organizations

  • University of Massachusetts Lowell

Tags

DTIC Thesaurus Topics

  • Abstracts
  • Assembly
  • Chemical Synthesis
  • Chemistry
  • Electrical Measurement
  • Enzymes
  • Films
  • Isotherms
  • Materials
  • Measurement
  • Molecules
  • Monomolecular Films
  • Polymerization
  • Polymers
  • Rocket Oxidizers
  • Self Assembly
  • Two Dimensional

Fields of Study

  • Chemistry

Readers

  • Molecular and Cellular Biochemistry
  • Organic Chemistry
  • Polymer Science and Engineering.