Excimers and Exciplexes of Conjugated Polymers

Abstract

Observations of intermolecular excimers in several pi-conjugated polymers and exciplexes of these polymers with tris(p-tolyl)amine are reported. It is shown that the luminescence of conjugated polymer thin films originates from excimer emission and that the generally low quantum yield is due to self-quenching. Thus in sufficiently dilute solution, the single-chain emission has a quantum yield of unity. Exciplex luminescence and exciplex-mediated charge photogeneration have much higher quantum yields than the excimer-mediated photophysical processes. These results provide a new basis for understanding and controlling the photophysics of conjugated polymers in terms of supramolecular structure and morphology.

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Document Details

Document Type
Technical Report
Publication Date
Jun 28, 1994
Accession Number
ADA281740

Entities

People

  • J0hn A. Osaheni
  • Samson A. Jenekhe

Organizations

  • University of Rochester

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Absorption
  • Charge Transfer
  • Chemical Engineering
  • Chemistry
  • Conjugated Polymers
  • Emission Spectra
  • Films
  • Luminescence
  • Materials
  • Molecules
  • Picosecond Time
  • Polymers
  • Quantum Yields
  • Solid Solutions
  • Spectra
  • Spectroscopy
  • Thin Films

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Nanocomposite Materials Science
  • Semiconductor Device Technology

Technology Areas

  • Quantum Computing