NLO Properties of Si(OH)4 and Ge(OH)4 Clusters
Abstract
The NLO properties in terms of static and frequency-dependent hyperpolarizabilities of Si(OH)4 and Ge(OH)4 clusters are determined with an aim to understand the microscopic NLO behavior of silica. The calculated results reveal that the cluster configuration induced by the presence of a defect plays a significant role in determining the non-linear response of these clusters. In addition, instant ionization of the cluster introduces a noticeable increase in the value of second hyperpolarizability gamma
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 01, 1994
- Accession Number
- ADA284514
Entities
People
- Michael Coolidge
- Ravindra Pandey
- Walter Lauderdale
Organizations
- Air Force Research Laboratory