Growth, Characterization and Application of KTN Family Nonlinear Optical Crystals.

Abstract

We have recently grown KLTN:(Cu, Ni, Ni/Ti) and SBT crystals and characterized their nonlinear-optical properties. The growth of these high quality crystals is a result of recent improvements in the crystal growth system; namely, improved flux uniformity and higher operating temperature. These and other materials have been characterized for application to holographic data storage and quasi-phase matched second harmonic generation. In particular, the paraelectric KLTN materials doped with Ni exhibit an enhanced long wavelength sensitivity (> 600 nm), which is desirable for recording holograms with ubiquitous He-Ne or semiconductor lasers. Furthermore, we have discovered that dynamic ferroelectric domain gratings in addition to the more common electrooptic gratings are present in SBN, a close relative of SBT. This has important applications to permanent fixing of volume holograms and tunable quasi-phase matching. To complement this experimental work, we have also derived analytical expressions for the two beam coupling process which allows us to deduce photorefractive material parameters for these crystals. This balance of experimental and theoretical work has enabled us to continually develop new materials whose properties are optimized for nonlinear optical applications.

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Document Details

Document Type
Technical Report
Publication Date
Nov 08, 1994
Accession Number
ADA290330

Entities

People

  • Amnon Yariv
  • Anthony Kewitsch
  • Rudy Hofmeister

Organizations

  • California Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Sensors

DTIC Thesaurus Topics

  • Barium Titanates
  • Chemical Compounds
  • Couplings
  • Crystal Growth
  • Crystals
  • Data Storage Systems
  • Electric Fields
  • Ferroelectric Domains
  • Holograms
  • Inorganic Chemicals
  • Long Wavelengths
  • Materials
  • Phase
  • Phase Diagrams
  • Photorefractive Materials
  • Space Charge
  • Transition Metals

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Optical Physics and Photonics.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics