Predictions of the Spectra of the Rare-Earth Ions Ce(3+) Through Yb(3+) in the Two Sites of Ca5(PO4)3F.

Abstract

The results of fitting the experimental data on Er(3+) in the two Ca2+ sites of Ca5(PO4)3F are used to predict the crystal-field parameters for the entire rare-earth series. These crystal-field parameters are then used along with the free-ion wavefunctions determined with aqueous parameters to determine a set of energy levels of the rare-earth ions Ce(3+) through Yb(3+) for both Ca(2+) sites (Cal with C(sub 3) symmetry and Ca2 with C(sub s) symmetry) in Ca5(PO4)3F. Also, the Judd-Ofelt parameters, Omega k are determined for each ion in the Cal and Ca2 sites, as well as the Zeeman g factors for the ground states. jg

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1995
Accession Number
ADA294471

Entities

People

  • Clyde A. Morrison

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Angular Momentum
  • Chemistry
  • Crystal Chemistry
  • Diffraction
  • Energy Levels
  • Equations
  • Experimental Data
  • Ground State
  • Lasers
  • Light Sources
  • Magnetic Dipoles
  • Optical Properties
  • Physics
  • Spectra
  • Spectroscopy
  • Symmetry
  • X Rays

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.