Exciton Dynamics in Poly(p-pyridyl Vinylene).

Abstract

We present results of picosecond photoinduced absorption (PA) and time resolved photoluminescence studies on solid and solution forms of poly(p-pyridyl vinylene). The nearly identical PA response of all forms of the polymer reflects the generation of the same primary photoexcitation, a Coulombically bound intrachain singlet exciton, and the absence of exotic species such as interchain excimers. The time dependence of the PA points to direct intersystem crossing as the origin of triplet excitons, ruling out generation of free carriers as a precursor to exciton formation.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1996
Accession Number
ADA305228

Entities

People

  • Darren D. Gebler
  • J. W. Blatchford
  • L. B. Lin
  • S. W. Jessen
  • Yuanyuan Wang

Organizations

  • Ohio State University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Chemistry
  • Conjugated Polymers
  • Crossings
  • Dye Lasers
  • Dynamics
  • Excitation
  • Excitons
  • Films
  • Liquid Dye Lasers
  • Military Research
  • Photoexcitation
  • Picosecond Time
  • Polymers
  • Spectra
  • Spin-Orbit Interaction

Readers

  • Molecular Photonics/Laser Physics
  • Polymer Science and Technology
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics