Nucleation Growth and Defect Engineering in Diamond Thin Films.

Abstract

We studied the chemical nature of the substrate and the role of buffer layers on nucleation and growth of diamond during chemical vapor deposition (hot-filament). The transition metals with partially filled d-atomic orbitals are found to stabilize SP2 bonding which leads to enhanced precipitation of SP2 bonded non-diamond carbon phases such as graphite, amorphous and glassy carbon films. We have shown that by alloying these metals with electron donating elements, it is possible to stabilize SP3 bonding and form diamond film directly on the metallic substrates. Similar studies on nucleation and growth of diamond have been performed using AlN buffer layers. The results from these studies are compared with those obtained using buffer layers. By using these concepts, we have minimized the formation of graphitic layers and improved the adhesion of diamond layers on non-carbide forming metallic substrates.

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Document Details

Document Type
Technical Report
Publication Date
Feb 01, 1996
Accession Number
ADA308255

Entities

People

  • Jagdish Narayan

Organizations

  • North Carolina State University

Tags

DTIC Thesaurus Topics

  • Atomic Orbitals
  • Bonding
  • Chemical Vapor Deposition
  • Coatings
  • Diamond Films
  • Engineering
  • Films
  • Materials
  • Materials Processing
  • Materials Science
  • Nucleation
  • Substrates
  • Thin Films
  • Transition Metals
  • Transitions
  • Vapor Deposition

Fields of Study

  • Materials science
  • Physics

Readers

  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space