Detailed Studies of Soot Formation in Laminar Diffusion Flames for Application to Modeling Studies.

Abstract

An investigation of soot formation in laminar diffusion flames showed that soot particle surface growth under laminar diffusion flame conditions ceases because of the depletion of hydrocarbon species and not soot particle reactivity loss due to thermal aging of the particles. This result was obtained through direct species concentration measurements under well-controlled conditions, while the particle reactivity effects were calculated based on premixed flame results along with particle temperature/time information available from earlier laminar diffusion flame studies. Comparisons with a soot formation model which incorporated detailed chemistry effects showed good agreement in terms of predicted and measured species concentration and soot particle field evolution. In addition, a novel technique for measuring soot volume fraction was developed based on laser-induced incandescence and was successfully applied to similar laminar diffusion flame studies. This technique was extended to droplet and turbulent diffusion flame conditions where a two-dimensional imaging approach was employed to measure soot volume fraction. Finally, the complete data set from these studies was assembled in a form suitable for dissemination on computer diskettes throughout the research community for comparison with modeling efforts.

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Document Details

Document Type
Technical Report
Publication Date
Jan 30, 1996
Accession Number
ADA310030

Entities

People

  • Robert J. Santoro

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • Biomedical
  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Air Force
  • Blackbody Radiation
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Combustion
  • Computers
  • Hydrocarbon Fuels
  • Measurement
  • Mechanical Engineering
  • Optics
  • Organic Chemistry
  • Reaction Mechanisms
  • Turbines
  • Turbulent Diffusion
  • Two Dimensional

Readers

  • Aerosol Science/Aerosol Physics
  • Combustion science or combustion engineering.
  • Computational Modeling and Simulation

Technology Areas

  • Directed Energy