Diagnostics of Diamond Film Deposition Plasmas.

Abstract

Diagnostic measurements of diamond-depositing dc arcjet plasmas are described. Polycrystalline diamond films with high-quality Raman spectra are grown using both low-pressure (5 to 40 Torr) and high-pressure (200 Torr) plasma arcjets. A number of different techniques, including laser-induced fluorescence (LIF), optical emission spectroscopy, mass spectroscopy, and Langmuir probe methods were developed and applied to measure properties of the plasma's physical and chemical environment as it deposits diamond on a surface. Low pressure arcjets are usually well out of thermal equilibrium even as they strike the substrate surface. LIF measurements show the gas temperature actually increases downstream of the arc, from 1800 to 2400 K, as a result of hydrogen atom recombination, whereas, Langmuir probe measurements show the electron temperature is roughly constant at 1 to 2 eV (12,000 to 24,000 K). Many species important for characterizing the physical environment have been detected with the optical methods (C2, CH, C3), and the mass spectroscopic measurements have focused on the species thought to be important for diamond growth (CH3 and C2H2).

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1996
Accession Number
ADA313765

Entities

People

  • Jay. B. Jeffries
  • Kenneth R. Stalder

Organizations

  • SRI International

Tags

Communities of Interest

  • Advanced Electronics
  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Chemical Reactions
  • Chemical Vapor Deposition
  • Chemistry
  • Diamond Films
  • Electrons
  • Energy Transfer
  • High Pressure
  • Laser Induced Fluorescence
  • Lasers
  • Mass Spectroscopy
  • Materials
  • Measurement
  • Military Research
  • Molecular Physics
  • Physics Laboratories
  • Spectra
  • Spectroscopy

Fields of Study

  • Physics

Readers

  • Plasma Physics.
  • Pulsed Power and Plasma Physics.
  • Thin Film Deposition Science.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Directed Energy - Pulsed-Laser Deposition
  • Fully Networked C3
  • Microelectronics
  • Microelectronics - Graphene