Photoinduced Electron Transfer in Binary Blends of Conjugated Polymers.

Abstract

We report observation of photoinduced electron transfer between two n-conjugated polymers in binary mixtures. Picosecond transient absorption and fluorescence spectroscopies of mixtures of n-type (electron accepting) poly (benzimidazobenzophenanthroline ladder) (BBL) and p-type (electron donating) poly (p- phenylene benzobisthiazole) (PBZT) or poly(p-(2-hydroxy)-phenylene berizobisoxazole) (HPBO) evidence intermolecular electron transfer when BBL is selectively photoexcited. The results suggest that blends of n-conjugated polymers are supramolecular materials which have novel features such as delocalized radical ion pairs or diion pairs, - novel properties, and- implications for organic p-n junction devices, photodiodes, photovoltaic cells, photoreceptors, and molecular electronic devices.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Sep 09, 1996
Accession Number
ADA314426

Entities

People

  • L. R. De Paor
  • R. M. Tarkka
  • S. A. Jenekhe
  • X. L. Chen

Organizations

  • University of Rochester

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Chemical Engineering
  • Chemistry
  • Conjugated Polymers
  • Detectors
  • Electron Transfer
  • Electronics
  • Electrons
  • Films
  • Macromolecules
  • Materials
  • Optical Properties
  • Polymers
  • Rigid Rod Polymers
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Molecular Photonics/Laser Physics
  • Polymer Science and Technology
  • Semiconductor Device Technology

Technology Areas

  • Directed Energy
  • Microelectronics