Silicon Etching and Growth Mechanisms via Ab Initio - Derived Surface Dynamics.

Abstract

In the enclosed report, Dr. E. A. Carter summarizes her accomplishments during the four years associated with this grant. These include developments of new numerical methods for accurate quantum mechanical descriptions of molecules and a new algorithm for finding transition states for chemical reactions. The majority of the effort expended by Carter's group, however, was related to semiconductor surface chemistry. She developed a synergistic approach, combining ab initio quantum chemistry to obtain accurate energetics and chemical rate constants, with ab initio molecular dynamics to follow reaction pathways on short time scales and Monte Carlo simulations to follow reactions on long time scales. This allowed her to gain insight into SiGe alloy superlattice structures, etching of Si by fluorine, the rate limiting chemical vapor deposition process of desorption of H2 from Si, and dissociative chemisorption of NH3 on Si.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1997
Accession Number
ADA325655

Entities

People

  • Emily A. Carter

Organizations

  • University of California, Los Angeles

Tags

Communities of Interest

  • Energy and Power Technologies
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Chemical Compounds
  • Chemical Engineering
  • Chemical Kinetics
  • Chemical Reactions
  • Chemistry
  • Density Functional Theory
  • Electronic Structure Theory
  • Kinetics
  • Molecular Dynamics
  • Perturbation Theory
  • Physical Chemistry
  • Potential Energy
  • Quantum Chemistry
  • Semiconductors
  • Simulations
  • Subatomic Particles
  • Surface Chemistry

Fields of Study

  • Materials science

Readers

  • Computational Modeling and Simulation
  • Quantum Chemistry
  • Semiconductor Device Technology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Quantum Computing