A Novel Photochemical Interfacial Approach to the Degradation of Hazardous Materials

Abstract

Two studies are described. The first involved the use of time resolved electron spin resonance as a mechanistic and spectroscopic probe of two fundamental reactions of ketone photochemistry: intermolecular hydrogen abstraction by the triplet state of benzophenone and triplet state alpha-cleavage of 1,3-diphenylacetone (dibenzyl ketone). It was found that the forces restricting the ground state conformations of these ketones also restrict the triplet state conformations. The second study used steady-state spectroscopies and laser flash photolysis techniques to define the mechanism involved in biologically and medicinally related compounds employed as anticancer agents and a compound called A2-E, a bis-retinoid found inocular cells, believed to be associated with age-related macular degeneration.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1997
Accession Number
ADA329694

Entities

People

  • Nicholas J. Turro

Organizations

  • Columbia University

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Antineoplastic Agents
  • Chemistry
  • Degradation
  • Diseases And Disorders
  • Electron Density
  • Electron Spin Resonance
  • Electrons
  • Ground State
  • Hazardous Materials
  • Ketones
  • Materials
  • New York
  • Photochemistry
  • Resonance
  • Retinal Diseases
  • Spin Resonance
  • Steady State

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Quantum Chemistry

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Microelectronics