Acquisition of a Scanning Ultrasound Analyzer for Gelation and Drying Studies in Sol-Gel Ceramic Coatings and Monoliths

Abstract

The overall goal of this research project was to develop a fundamental understanding of how colloid chemistry influences structure and properties of ceramic monoliths fabricated by sol-gel synthesis from colloid suspensions. The specific objective in the first part of the project was to determine how the interaction potential between colloidal particles influenced gel structure and strength. We proposed to do this using Stokesian Dynamics computer simulations and time-dependent ultrasonic measurements of elastic modulus for gels synthesized using various colloidal silica sol concentrations and electrolyte strengths. Detailed negotiations about equipment pricing and capabilities revealed that a simpler experimental method (mechanical rheometry) could be more effective than the proposed ultrasonic technique for elucidating time-dependent gel structure evolution and yielding. With the written permission of Dr. Pechenik, the Program Director, funding allocated for purchasing the ultrasonic device and designated matching funds from Texas A&M University were used to purchase a Paar Physica Universal Dynamic Spectrometer (UDS). During the last year this instrument was successfully purchased installed at Texas A&M University and is already shedding needed light on the gelation kinetics of concentrated colloid suspensions. The following report summarizes our reasons for choosing the UDS and provides an overview of our research findings using the instrument.

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1997
Accession Number
ADA332635

Entities

People

  • Lynden A. Archer

Organizations

  • Texas A&M University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Acquisition
  • Analyzers
  • Ceramic Coatings
  • Chemical Engineering
  • Chemistry
  • Coatings
  • Computer Simulations
  • Computers
  • Dynamics
  • Electrolytes
  • Gelation
  • Kinetics
  • Materials
  • Measurement
  • Modulus Of Elasticity
  • Simulations
  • Universities

Readers

  • Aerosol Science/Aerosol Physics
  • Surface Coatings Technology.
  • Theoretical Analysis.