Transformation Weakening of Ceramic Composite Interfaces

Abstract

A new concept for achieving graceful failure in oxide composites is studied. It is based on debonding of a weak interphase between a matrix and an interphase in a laminated composite. The interphase can be thermally or shear stress induced by transformation weakening, which results from an accompanying significant volume contraction and/or unit cell shape change, on cooling from a high temperature to low temperature crystal structure. Mullite/cordierite laminates with a beta --> alpha-cristobalite transformation weakened interphase were investigated in order to demonstrate interphase debonding behavior. The laminate showed fracture behavior dependent on a critical size effect. The grain size of polycrystalline beta-cristobalite was controlled by annealing. With increasing annealing time, the strength decreased due to the formation of internal microcracks in the cristobalite layer which occurred spontaneously during thermally-induced transformation. A hot-pressed laminate, annealed for 10 h at 1300 deg C, had an average grain size of 4.2 micrometers and a strength of 131 MPa. Its work of fracture was 2.38 kJ/sq m with a non-catastrophic fracture behavior. The indentation response indicated crack deflection along the cristobalite debonding interphase.

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Document Details

Document Type
Technical Report
Publication Date
Oct 31, 1997
Accession Number
ADA334604

Entities

People

  • Waltraud M. Kriven

Organizations

  • University of Illinois Urbana–Champaign

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Ceramic Materials
  • Ceramic Matrix Composites
  • Chemical Synthesis
  • Chemistry
  • Composite Materials
  • Crystal Structure
  • Crystals
  • Laminates
  • Material Degradation Processes
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Mechanics
  • Phase Transformations
  • Structural Ceramics

Readers

  • Powder metallurgy of Titanium alloys.
  • Reinforced Composite Materials