Rapid Concentration Measurements by Picosecond Time-Resolved Laser-Induced Fluorescence

Abstract

Quantitative measurements of scalars in combustion are crucial to our understanding of flame structure and pollutant production. Progress has been made in quantitatively characterizing many laminar flames; however, the inherent fluctuations in turbulent flames significantly complicate such measurements. Picosecond time-resolved laser-induced fluorescence (PITLIF) is a developing technique which seeks to provide the first known means of obtaining quantitative minor-species concentrations in flames at rates sufficient for the study of turbulent fluctuations. This method was developed and applied to measurements of sodium and OH concentrations in laminar flames under previous AFOSR funding. The present report details the construction of a second generation PITLIF instrument. The primary goal of this work is to provide a continuous time series of quantitative concentrations from which frequency domain statistics such as the power spectral density (PSD) can be computed. Using the new laser system, fluorescence measurements of CH and OH time series were collected in a variety of methane and hydrogen flames including nonpremixed turbulent flames. These data have also been compared with available velocity and temperature measurements. The time series and resulting PSDs represent the first measurements of these statistics for minor-species concentrations.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Apr 03, 1998
Accession Number
ADA342577

Entities

People

  • G. B. King
  • N. M. Laurendeau

Organizations

  • Purdue University

Tags

Communities of Interest

  • Energy and Power Technologies
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Amplifiers
  • Chemical Reactions
  • Chemistry
  • Convection
  • Dye Lasers
  • Fluorescence
  • Frequency
  • Hydrogen
  • Laser Applications
  • Laser Beams
  • Laser Induced Fluorescence
  • Lasers
  • Measurement
  • Picosecond Time
  • Reynolds Number
  • Turbulent Diffusion
  • Turbulent Mixing

Fields of Study

  • Physics

Readers

  • Atmospheric Science / Meteorology, specifically Wind Wave Turbulence.
  • Combustion science or combustion engineering.

Technology Areas

  • Directed Energy