Processes Affecting Reductive Dechlorination of Chlorinated Solvents by Zero-Valent Iron

Abstract

Zero-valent iron may participate in the reductive dechlorination process by three different mechanisms: direct, electrolytic reduction; reduction by hydrogen produced during the corrosion process; and reduction by dissolved (ferrous) iron that is also produced by corroding iron. The first step of electrolytic reduction is presumably, the transfer of one electron from the metal surface to the organic molecule. This results in an organic anion radical that may then lose a halide anion to give a carbon-centered radical, and oxidized iron, which is eventually released to the solution as Fe(2+). The goal of our research is to provide a comprehensive survey of the mechanisms that affect the performance of this reactive barrier technology.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1993
Accession Number
ADA351154

Entities

People

  • Leah J. Matheson
  • Paul G Tratnyek

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Abstracts
  • Carbon Tetrachloride
  • Chemical Synthesis
  • Chemistry
  • Chlorinated Hydrocarbons
  • Classification
  • Copyrights
  • Corrosion
  • Ecology
  • Electrons
  • Engineering
  • Halogenated Hydrocarbons
  • Hydrocarbons
  • Hydrogen
  • Information Operations
  • Molecules
  • United States

Fields of Study

  • Chemistry

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  • Groundwater Contamination Remediation.
  • Materials Science and Engineering.
  • Organic Chemistry

Technology Areas

  • Microelectronics