Anticancer Agents Based on a New Class of Transition- State Analog Inhibitors for Serine and Cysteine Proteases.

Abstract

In this report we describe our efforts to develop a new class of competitive inhibitors for serine and cysteine proteases. These compounds are potential anticancer agents that would act by inhibiting metastasis and angiogenesis. The first part of this report describes solution and solid phase methods for the synthesis of inhibitors of the cysteine protease cathepsin B. These inhibitors are based on a cyclohexanone pharmacophore and are designed to interact with both the S and S' subsites of the enzyme active site. In the second part we demonstrate that the 4-heterocyclohexanone pharmacophore can be used to synthesize effective inhibitors of serine proteases. We have constructed an inhibitor of the serine protease plasmin, and shown that it has good activity and significant specificity for plasmin over other proteases.

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1998
Accession Number
ADA355419

Entities

People

  • Chrchristopher T. Seto

Organizations

  • Brown University

Tags

DTIC Thesaurus Topics

  • Alkenes
  • Amino Acids
  • Antineoplastic Agents
  • Cancer
  • Carboxylic Acids
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Crystal Structure
  • Cyclohexanones
  • Diseases And Disorders
  • Ketones
  • Materials
  • Neoplasms
  • Organic Chemistry
  • Solid Phases

Fields of Study

  • Chemistry

Readers

  • Molecular and Cellular Biochemistry