Overcharge Protection in Ambient Temperature Lithium and Lithium-Ion Cells: A Literature Survey

Abstract

This report summarizes a survey of the literature on in situ electrochemical methods to provide overcharge protection in ambient temperature lithium and lithium-ion cells. Among the various rechargeable lithium battery systems, only the lithium cells using solutions of inorganic salts such as LiAlCl4 or LiGaCl4 in sulfur dioxide as electrolytes were found to have inherent overcharge protection. For low-voltage lithium cells such as lithium/titanium disulfide, the survey identified a number of electrolyte additives that undergo oxidation above the charging potentials but below the solvent oxidation potential and can provide overcharge protection in these cells. The oxidized form of the additive then reacts with lithium to regenerate the original electrolyte additive. However, no suitable electrochemical method was identified for providing overcharge protection in lithium or lithium-ion cells that require charging to potentials above approx. 4 V.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1998
Accession Number
ADA359152

Entities

People

  • Wishvender K. Behl

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • Aromatic Compounds
  • Carbonate Esters
  • Carbonates
  • Dielectric Gases
  • Lead Acid Batteries
  • Literature Surveys
  • Lithium Batteries
  • Lithium Ion Batteries
  • Low Voltage
  • Metal Oxides
  • Metallocenes
  • Military Research
  • Nickel Cadmium Batteries
  • Organic Compounds
  • Oxidation
  • Oxides
  • Storage Batteries

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Organic Chemistry