Multi-Stage Selective Catalytic Reduction of NOx in Lean-Burn Engine Exhaust

Abstract

Recent Studies suggest that the conversion of NO to NO2 is an important intermediate step in the selective catalytic reduction (SCR) of NOx to N2. These studies have prompted the development of schemes that use an oxidation catalyst to convert NO to NO2, followed by a reduction catalyst to convert NO2 to N2. Multi-stage SCR offers high NOx reduction efficiency from catalysts that, separately, are not very active for reduction of NO, and alleviates the problem of selectivity between NO reduction and hydrocarbon oxidation. A plasma can also be used to oxidize NO to NO2. This paper compares the multi-stage catalytic scheme with the plasma-assisted catalytic scheme for reduction of NOx in lean-burn engine exhausts. The advantages of plasma oxidation over catalytic oxidation are presented.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1997
Accession Number
ADA363496

Entities

People

  • B. M. Penetrante
  • B. T. Merritt
  • G. E. Vogtlin
  • M. C. Hisao

Organizations

  • Lawrence Livermore National Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Catalysis
  • Catalysts
  • Catalytic Oxidation
  • Chemistry
  • Diesel Engines
  • Efficiency
  • Electric Power
  • Engines
  • Exhaust Gases
  • Gases
  • Governments
  • Hydrocarbons
  • Internal Combustion Engines
  • Materials
  • Oxidation
  • United States Government
  • Workshops

Fields of Study

  • Chemistry
  • Environmental science

Readers

  • Applied Combinatorial Optimization and Logic Circuit Design.
  • Combustion science or combustion engineering.
  • Molecular and Cellular Biochemistry