New Theories for Erosion-Corrosion

Abstract

The erosion-corrosion of copper and copper-nickel alloys in synthetic seawater was investigated using an impinging jet. Video microscopy, corrosion potential monitoring, and impedance spectroscopy were used to investigate the state of the system and the reactivity of the electrode surface. Shear-induced removal of salt films was observed and found to be associated with significant increases in surface reactivity. Direct shear-induced removal of oxide films, however, was not observed. Nevertheless, the protective oxide layer showed sensitivity in passively aerated seawater to large fluid velocities and to small perturbations in potential. The films were stable under all conditions tested in continuously aerated seawater. The present work supports the argument that localized corrosion of copper alloys is caused by galvanic coupling between different regions of a metal coupon. Thus, cathodic protection may be used to prevent such corrosion. A modeling and experimental study was conducted to show the conditions under which non-uniform current distributions influence the impedance response of a disk electrode. Measurement model tools were developed to identify the stochastic and experimental bias errors. This information was used to filter data, design experiments, and assess the validity of regression assumptions and the confidence intervals of the resulting parameters.

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Document Details

Document Type
Technical Report
Publication Date
Jun 05, 1999
Accession Number
ADA364887

Entities

People

  • Mark E. Orazem

Organizations

  • University of Florida

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Chemical Engineering
  • Chemical Kinetics
  • Chemical Synthesis
  • Chemistry
  • Computational Science
  • Cyanides
  • Differential Equations
  • Diffusion Coefficient
  • Electrical Circuits
  • Electrochemistry
  • Experimental Design
  • Mass Transfer
  • Materials
  • Materials Processing
  • Materials Science
  • Measurement
  • Physical Properties

Readers

  • Computational Modeling and Simulation
  • Electrochemical Surface Science
  • Materials Science and Engineering.