Fluorescence Image of a Single Molecule in a Microsphere: Model

Abstract

We model fluorescence images of single molecules in spherical dielectric microcavities. Molecules are treated as time-harmonic dipoles. Images are integrated over emission frequencies. Because of the strong refractive properties of the enclosing sphere, the fluorescence image depends on the refractive index of the sphere and the position, orientation, and emission frequency of the molecule. When the dipole's emission is at the frequency of a microsphere resonance, the brightest regions in the images appear to originate from outside the sphere for some dipole positions. This type of calculation should help in interpreting images of molecules in microspheres.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1999
Accession Number
ADA367750

Entities

People

  • J. M. Ramsey
  • Michael D. Barnes
  • Paul Nachman
  • Stephen Arnold
  • Steven C. Hill

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Coordinate Systems
  • Diffraction
  • Elastic Scattering
  • Emission
  • Fluorescence
  • Frequency
  • Geometric Forms
  • Microspheres
  • Military Research
  • Molecules
  • Orientation (Direction)
  • Refractive Index
  • Resonance
  • Resonant Frequency
  • Scattering
  • Spheres
  • Spherical Waves

Fields of Study

  • Physics

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Electromagnetic Wave Scattering and Antenna Radiation Engineering
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.