Solid-State Thermochemistry of Flaming Combustion

Abstract

The thermal and chemical processes which occur in the solid state during flaming combustion are examined. A phenomenological model of fuel generation provides the relationships between macroscopic flammability parameters and polymer chemical structure and shows how the coupling of thermal diffusion and chemical kinetics occurs naturally in the pyrolysis zone. Fire behavior and flammability of solid polymers are predicted using the ignition temperature, heat of combustion, heat of gasification, and char yield calculated from the chemical structure; and the results are compared to experimental values. The objective of this work is to develop a consistent, solid-state physical chemistry of flaming combustion which bridges the gap between fire and material sciences to help guide the discovery of new, more fire-resistant polymers.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1999
Accession Number
ADA367981

Entities

People

  • Richard E. Lyon

Organizations

  • Federal Aviation Administration

Tags

Communities of Interest

  • Biomedical
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Biomedical And Dental Materials
  • Burning Rate
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Combustion
  • Heat Transfer
  • Material Degradation Processes
  • Materials Laboratories
  • Materials Science
  • Materials Testing
  • Plastics
  • Polymer Chemistry
  • Polymer Degradation
  • Polymeric Films
  • Thermodynamics

Readers

  • Materials Science and Engineering.
  • Petroleum Engineering
  • Thermal Physics or Thermal Science.