Diode-Pumped Nd:YAG/Cr(4+):YAG MicroChip-Laser System at 214.8 nm for the Detection of NO

Abstract

A passively Q-switched 214.8-nm Nd:YAG/Cr(4+):YAG microchip-laser system for the detection of NO was designed, constructed, and tested. The system uses the fifth harmonic of the 1.074-micrometers transition in Nd:YAG to detect NO at the few-parts-per-billion level. A significant challenge was the development of an environmentally stable coating to provide the necessary discrimination between the 1.074-micrometers laser line and the stronger transition at 1.064 micrometers. The exact position of the fifth-harmonic frequency was determined using NO fluorescence excitation spectra to be 46556/cm. We observed a detection sensitivity for NO of about 15 ppb(v) in a simple, compact optical system. Earlier observations of SO2 imply a similar or better sensitivity for the current system, while green-light excitation of NO2 fluorescence yielded a detection limit of order 1 ppm(v). Applications of the laser system described here include explosives sensors based on detection of NO from thermal decomposition, and NO(x)/SO(x) monitors for trucks, aircraft and stationary sources.

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Document Details

Document Type
Technical Report
Publication Date
Jul 30, 1999
Accession Number
ADA370924

Entities

People

  • C. Cook
  • J. H. Shorter
  • J. Wormhoudt
  • J.j. Zayhowski

Organizations

  • Aerodyne Research

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Human Systems
  • Sensors

DTIC Thesaurus Topics

  • Absorption Coefficients
  • Data Acquisition
  • Detection
  • Detectors
  • Explosives
  • Explosives Detection
  • Fluorescence
  • Frequency
  • Laser Induced Fluorescence
  • Lasers
  • Measurement
  • Observation
  • Optical Materials
  • Photomultiplier Tubes
  • Repetition Rate
  • Spectra
  • Transitions

Fields of Study

  • Physics

Readers

  • Analytical Chemistry
  • Optical Fiber Sensing and Electromagnetic Propagation.
  • Pulsed Power and Plasma Physics.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers