Steady-State Potential Scan at Rotating Disk Electrode and Applications

Abstract

A method of multiple small potential steps was applied to obtain current-potential curves at a rotating disk electrode (RDE), which is more accurate than the classical potential scan RDE method. Several basic benefits of the new RDE method were summarized, including reducing charging current, removing adsorption current, identifying kinetic current, and separating kinetic and diffusion reactions. The practical application of this new method is to study high-surface-area powder catalysts for fuel cell research. An example of using this new method was demonstrated by measurement of the current-potential curves of catalytic oxygen reduction on a heat-treated, metalloporphyrins-coated graphite RDE. A successful kinetic analysis of catalytic oxygen reduction at the powder-catalyst-coated electrode was achieved.

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 2000
Accession Number
ADA382650

Entities

People

  • Charles Walker
  • Deryn Chu
  • Rongzhong Jiang

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Adsorption
  • Alcohols
  • Catalysis
  • Catalysts
  • Cells
  • Diffusion
  • Diffusion Coefficient
  • Electrochemical Reactions
  • Electrodes
  • Equations
  • Fuel Cells
  • Kinetics
  • Materials
  • Measurement
  • Military Research
  • Sorption
  • Steady State

Fields of Study

  • Environmental science

Readers

  • Organic Chemistry
  • Systems Analysis and Design
  • Thin Film Deposition Science.

Technology Areas

  • Biotechnology