Templated Grain Growth of Single Crystal-Like Electroceramics

Abstract

Fiber textured bismuth titanate (Bi4Ti3O12) (BIT) and biaxially textured La-doped Sr2Nb2O7 (SN) were produced by templated grain growth. Platelets of BIT and blade-shaped SN template particles were dispersed in a matrix of nanosize BIT and fine SN powders, respectively. and aligned by tape casting. As determined by x-ray diffraction and microscopy. the sintered ceramics were >90% textured. Growth of the template particles depends critically on the presence of a liquid during growth and maintaining a template to matrix grain size ratio >2. Textured Nb-doped bismuth titanate ceramics (Bi4Ti(3-x/5)Nb(x/5)O12. where x=0.02) showed anisotropic dielectric and piezoelectric properties when measured parallel and perpendicular to the texture axes with the remanent polarization differing by more than a factor of 15 in the two directions. The piezoelectric constant in the grain-axis was 30 pC/N. or ^77% of the single crystal value. High temperature piezo, doped bismuth titanate. A gated doctor blade was developed to achieve biaxial alignment of the blade-shaped Sr2Nb2O7 template particles. Very good orientation was achieved perpendicular to the major blade axis In addition, X-ray diffraction measurements of the 131 pole revealed that the Sr2Nb2O7 was biaxially textured and had a full width at half maximum of the peak height of 30 deg in the orientation distribution in the plane of the blades.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2001
Accession Number
ADA386724

Entities

People

  • Gary L. Messing
  • Susan Trolier-McKinstry

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms

DTIC Thesaurus Topics

  • Bismuth Titanate
  • Ceramic Materials
  • Chemistry
  • Crystals
  • Dielectric Properties
  • Epitaxial Growth
  • Grain Growth
  • Grain Size
  • High Temperature
  • Materials
  • Materials Science
  • Measurement
  • Orientation (Direction)
  • Particles
  • Single Crystals
  • Titanates
  • X-Ray Diffraction

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.