Cycle Life Enhancement in Cu-Sn Anodes

Abstract

This technical report summarizes the work on two different approaches that have been used to increase the cycle life of active-inactive composites in the copper-tin system. The first approach is to reduce the particle size of the active-inactive composities to the nano-scale (< 100 nm). The second approach is the addition of extra elements that segregate to grain/phase boundaries and increase the cohesive strength of the boundary. Both approaches significantly improved the capacity retention of a Cu6Sn5 alloy. A larger improvement in capacity retention was exhibited by the addition of 10-wt.% iron compared to the reduction of the particle size to the nano-scale. The volumetric capacity of the Cu6Sn5 alloy containing 10 wt. % iron at 100 cycles is almost three times the theoretical capacity of graphite. The Cu6Sn5-10 wt.% Fe material has potential as a replacement anode for graphite in lithium-ion batteries.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 2002
Accession Number
ADA403236

Entities

People

  • Donald Foster
  • Jeff Wofenstine
  • Jeffrey Read
  • Wishvender Behl

Organizations

  • United States Army Research Laboratory

Tags

DTIC Thesaurus Topics

  • Alloys
  • Boundaries
  • Composite Materials
  • Diffraction
  • Electron Microscopy
  • Elements
  • Grain Boundaries
  • Graphitic Materials
  • Lithium Ion Batteries
  • Materials
  • Military Research
  • Particle Size
  • Particles
  • Resistance
  • Transmission Electron Microscopy
  • X Rays
  • X-Ray Diffraction

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Powder metallurgy of Titanium alloys.