Block Copolymer-Based Thermoset Nanocomposites

Abstract

Amphiphilic block copolymers have been added to two-part epoxy resin and cured leading to well-defined nanocomposites. Reactive and non-reactive polar blocks were coupled to non-polar hydrocarbon blocks using anionic and living free-radical polymerization techniques. Mixtures containing 0 to 100% block copolymer were investigated for structure by small-angle X-ray scattering and transmission electron microscopy, and for mechanical properties by compact tension testing. Spherical micelles and vesicles were documented at low block concentrations, and these nanocomposites exhibit enhanced fracture toughness. Chemical bond formation between the matrix and block copolymer leads to some improvement in toughness.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Feb 01, 2002
Accession Number
ADA403744

Entities

People

  • Frank S. Bates

Organizations

  • University of Minnesota

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Biomedical And Dental Materials
  • Block Copolymers
  • Chemical Engineering
  • Chemistry
  • Copolymers
  • Electron Microscopy
  • Epoxy Resins
  • Free Radicals
  • Materials
  • Materials Science
  • Mechanical Properties
  • Modulus Of Elasticity
  • Nanocomposites
  • Plastics
  • Polymers
  • Resins
  • Thermosetting Plastics

Fields of Study

  • Materials science

Readers

  • Nanocomposite Materials Science
  • Polymer Science and Technology

Technology Areas

  • Microelectronics