Design, Synthesis and Evaluation of Organic Non-linear Optical Chromophores with Configurationally and Conformationally Locked Polyene Bridges

Abstract

A modular, synthetic scheme was developed for versatile variation of donors, acceptors and polyene bridge length of NLO-chromophores. Configurational- and conformational rigidity of the polyene bridges were realized by making each set of adjacent double and single bond pair part of a fused cylohexene ring. Substituent effects on the reactions leading to the establishment of the donor, elongation of the fused polyene bridge and the final introduction of the acceptor moiety were uncovered and used to control regioselectivity, chemo-selectivity and reactivity in the overall synthetic scheme.

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Document Details

Document Type
Technical Report
Publication Date
Sep 30, 2002
Accession Number
ADA407110

Entities

People

  • Godson C. Nwokogu
  • Samuel A. Simpson

Organizations

  • Hampton University

Tags

DTIC Thesaurus Topics

  • Acids
  • Alkenes
  • Chemical Synthesis
  • Chemistry
  • Chromophores
  • Condensation
  • Cyclohexenes
  • Elongation
  • Esters
  • Low Temperature
  • Materials
  • Methylenes
  • Organic Chemistry
  • Reactivities
  • Test And Evaluation
  • Thiobarbituric Acid

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Organic Chemistry
  • Parasitology and Pharmacology of Malaria.