Atomic Lithography: Forcing Epitaxial Growth Using X-ray Standing Waves

Abstract

Over the last year we made considerable progress towards demonstrating an effect of an x-ray standing wave on the deposition of a Ge film. In the presence of the standing wave we observed a change in the film morphology of Ge grown on Si(111) below the temperature needed for epitaxial growth. Beam-exposed regions appear flat and resemble the Si(111) substrate, while unexposed regions are rough and display polycrystalline morphology similar to that seen for Ge growth on amorphous substrates. Consistent with our expectations, at higher deposition temperatures the effect is no longer observable. Similarly, for the deposition conditions we have been able to investigate to date on amorphous substrates we do not see any difference in the morphology between beam-on and beam-off regions. This is consistent with an effect arising from a weak coupling between the standing wave field and the Ge atoms on the surface which, at the x-ray intensities we can achieve without modifications to our optical geometry, is insufficient to modify the growth by itself, but when coupled with the periodic potential due to the substrate can push the Ge atoms into a new stable configuration. We found this to be very promising development toward our ultimate goal of atomic lithography. Below, we discuss in more detail the experimental approach to these recent standing wave depositions and their results.

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Document Details

Document Type
Technical Report
Publication Date
Nov 06, 2002
Accession Number
ADA408986

Entities

People

  • Charles M. Falco

Organizations

  • University of Arizona

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Couplings
  • Crystals
  • Detectors
  • Epitaxial Growth
  • Geometry
  • Intensity
  • Lithography
  • Polycrystals
  • Radiation
  • Reflectors
  • Standing Waves
  • Substrates
  • Surface Properties
  • Temperature Gradients
  • Transition Temperature
  • Waves
  • X Rays

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Nanofabrication and Microfabrication.
  • Systems Analysis and Design