The Synthesis and Characterization of Methylene Bisoxyamine CH2(-O-NH2)2 Salts

Abstract

A large family of energetic salts were made using methylene bisoxyamine, CH2(-O-NH2)2, a dibasic, geminal oxyamine of methane. Single salts including the nitrate, perchlorate, dinitramide, and nitroformate, and doubly protonated methylene bisoxyamine salts, nitrate, perchlorate and bisdinitramide, were all synthesized in good to high yields, from simple acid-base reactions with the corresponding aci-forms of energetic anions. All of the salts were characterized by vibrational (IR, Raman), multinuclear nmr (1H, 13C), and DSC studies. The single crystal X-ray diffraction study was carried out on the double perchlorate salt. Initial safety studies (impact and friction), were carried out on most of the new materials, as well as the thermal stability of these salts at 75 deg C.

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Document Details

Document Type
Technical Report
Publication Date
Feb 14, 2001
Accession Number
ADA409718

Entities

People

  • Adam Brand
  • Greg Drake
  • Kerri Tollison
  • Milton Mckay
  • Tom Hawkins

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force Research Laboratories
  • Alcohols
  • Chlorides
  • Energetic Materials
  • High Vacuum
  • Infrared Spectra
  • Materials
  • Military Research
  • Propellants
  • Raman Spectra
  • Solid Propellants
  • Solid Rocket Oxidizers
  • Spectra
  • Spectroscopy
  • Thermal Stability
  • Vibrational Spectra
  • X-Ray Diffraction

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry