Solid Phase Combinatorial Approach to Estradiol Tamoxifen/Raloxifene Hybrids: Novel Chemotherapeutic/Prophylactic Selective Estrogen Receptor Modulators

Abstract

The objective of this project is the development of new chemotherapeutic agents for the treatment of hormone-responsive breast cancer using a solid phase approach to synthesize new agents having features common to both steroids and antiestrogens. Previously we functionalized the carboxy resin with both the E-and Z-tributylstannylvinyl estradiol, and prepared an initial series of iodophenoxyalkylamines that will be coupled to the resin-bound steroid. Coupling reactions with the Z-stannylvinyl estradiol were generally unsuccessful on solid-phase and coupling with the E-isomers proceeded in low yields. We have prepared more iodophenoxyalkylamines and are preparing the target compounds via solution phase methods. We are exploring an approach using resin-bound estradiol vinylboronic acids as an alternative method.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2002
Accession Number
ADA410893

Entities

People

  • Robert N. Hanson

Organizations

  • Northeastern University

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Abstracts
  • Alkenes
  • Assays
  • Bioassay
  • Biomedical Research
  • Boron Compounds
  • Breast Cancer
  • Chemical Compounds
  • Chemical Synthesis
  • Chemistry
  • Couplings
  • Estrogens
  • Modulators
  • Molecular Dynamics
  • Phase
  • Solid Phases
  • Test And Evaluation

Fields of Study

  • Chemistry

Readers

  • Breast cancer cell signaling and growth regulation.
  • Molecular and Cellular Biochemistry