Prediction of Advanced Nitramine Propellant Burning Rates with the CYCLOPS Code

Abstract

The ability to predict the burning rate of a propellant from its ingredients would be an extremely valuable aid to the formulation of new propellants. We have been developing such a capability over the last 5 years and recently described its use for nitrate-ester propellants. In this report, we first present results of applying this model (the CYCLOPS code) to advanced nitramines propellants, both cyclotrimethyeletrinitramine (RDX) and hexanitrohexaazaisowirtzitane (CL20) oxidizers in an energetic binder made of a bisazidomethylene oxetane-azidomethylenemethyl oxetane (BAMO-AMMO) mixture. A substantial revision in the available gas-phase reaction mechanism previously used for neat RDX was required, necessitating Quantum-Rice. Ramsperger-Kassel calculations for many new reaction paths. The resulting mechanism grew from 45 species and 232 reversible elementary reactions to 80 species and 550 revemible elementary reactions. Burning rates computed by the model compared very well with measured rates for both the RDX- and CL20-based propellants. Temperature profile measurements were available for the RDX propellant only, but the code computations indicated a much shorter dark zone than that measured with microthermocouples. These are the first calculations of burning rates for advanced nitramine propellants, and the results are encouraging.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2003
Accession Number
ADA416019

Entities

People

  • Martin S. Miller
  • William R. Anderson

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • Burning Rate
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemistry
  • Combustion
  • Decomposition
  • Double Base Propellants
  • Energetic Materials
  • Materials
  • Materials Laboratories
  • Materials Science
  • Measurement
  • Military Research
  • Nitramines
  • Propellants
  • Quantum Chemistry
  • Reaction Mechanisms

Fields of Study

  • Physics

Readers

  • Computer Programming and Software Development.
  • Rocket Propulsion.

Technology Areas

  • Quantum Computing