Environmental Impact of New Chemical Agents for Fire Suppression

Abstract

The environmental impact of chemical agents is intimately tied to the environmental transformations these chemicals undergo. In this project, the most important transformations for various classes of proposed fire suppression agents were investigated and, for the important case of hydrogen abstraction by hydroxyl radicals, a computational screening tool was developed. Rate constants for hydroxyl radical reactions with hydrofluoroethers, perfluoronated alkenes, bromine-containing fluoroalkenes, and fluoroalkanes, were determined. By using the computational tool developed in the project, rate constants and atmospheric lifetimes for several bromine-containing halomethanes were calculated. In addition, the reactivity of several alkyl phosphates with free radicals in water were measured and the solubility of a series of fluoroalkylamines was calculated.

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Document Details

Document Type
Technical Report
Publication Date
Aug 28, 2003
Accession Number
ADA418320

Entities

People

  • Robert E. Huie

Organizations

  • United States Army Corps of Engineers

Tags

Communities of Interest

  • Counter WMD
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alkanes
  • Alkenes
  • Chemical Compounds
  • Chemical Kinetics
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemical Warfare Agents
  • Chemistry
  • Computational Science
  • Environment
  • Ethers
  • Free Radicals
  • Geometry
  • Halogenated Hydrocarbons
  • Jet Propulsion
  • Organic Chemistry

Fields of Study

  • Chemistry
  • Environmental science

Readers

  • Fire Suppression Systems Design.
  • Molecular Photonics/Laser Physics
  • Organic Chemistry