Analysis of Keratin Filament Assembly/Disassembly and Structure Following Modification by Sulfur Mustard Analogs

Abstract

Characterization of vimentin intermediate filament (IF) structure by site directed spin labeling (SDSL) and electron paramagnetic resonance (EPR) has produced new data concerning the All arrangement of molecules in intact filaments. In the All alignement, rod 1B of a dimer is aligned with rod 1B of a second dimer. Our EPR data identify vimentin position 190 as the midpoint of overlap between dimers in the A11 arrangement. In conjunction with previously published data, we have thus identified contact surfaces between individual amino acids of rod 1B and rod 2B, involved in assembly of IFs. Analysis of keratin filament assembly and disassembly following treatment with the vesicant analogs 2-chloroethyl ethyl sulfide (CEES) and mechlorethamine (MEC) has been performed with 2 keratin pairs, one bacterially produced and one isolated from bovine tissue. Experiments with bacterially produced keratin 8 and 18 show that Intermediate Filaments assembled in vitro and subsequently treated with CEES and MEC are severely altered. The normal filament network is destroyed, replaced by aggregates of material with an irregular appearance. Experiments with k5 and k14 isolated from bovine tissue reveal the same results; CEES and MEC treatment destroy the smooth filamentous appearance of normal IFs and result in large aggregates.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 2003
Accession Number
ADA418634

Entities

People

  • John F. Hess

Organizations

  • University of California

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Amino Acids
  • Assembly
  • Cellular Structures
  • Chemical Synthesis
  • Chemical Weapons
  • Chemistry
  • Crystal Structure
  • Cytoskeleton
  • Disassembly
  • Electron Paramagnetic Resonance
  • Materials
  • Medical Personnel
  • Paramagnetic Resonance
  • Proteins
  • Resonance
  • Vesicants
  • Weapons

Readers

  • Analytical Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.
  • Reinforced Composite Materials

Technology Areas

  • Microelectronics