Development of Novel Process for the Deposition of Nanostructured Ternary Alloys and Composites for Replacement of Cadmium Coatings

Abstract

The objective of this investigation was to develop novel processes for depositing ternary Zn-Ni-X (X=Cu or P) alloys for replacement of Cd coatings in sacrificial protection of steel substrates. Introducing small amounts of Cu in the Zn-Ni plating bath results in alloys with reduced amount of Zn in the final deposit. This alloy shows improved corrosion performance that is 4 times higher than that of Cd coatings. Also, the use of autocatalytic method was investigated to deposit amorphous Ni-Zn-P alloys. The electroless Ni-Zn-P alloy shows improved corrosion performance that is 5 times higher than that of Cd coatings and reduces the hydrogen ingress into steel to 94%. A novel electrolytic process was developed to deposit Ni-Zn alloys with high Ni content. Deposition parameters like pH and temperature were optimized based on composition and the surface morphology of the coating. The Zn content in the coating was optimized based on the corrosion resistance of the final deposit. Finally. corrosion studies shows that Ni-Zn coatings obtained using these methods show a 5 times increase in barrier resistance as compared to Cd coatings. Also a mathematical model was developed to study the electroless Ni-Zn-P deposition.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 2003
Accession Number
ADA419640

Entities

People

  • Branko N. Popov

Organizations

  • University of South Carolina

Tags

Communities of Interest

  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Chemistry
  • Coatings
  • Corrosion
  • Corrosion Resistance
  • Electrodeposition
  • Electrolytic Processes
  • Elements
  • Fungi
  • Hydrogen
  • Hydrogen Embrittlement
  • Linear Polarization
  • Mass Transfer
  • Materials
  • Mathematical Models
  • Mechanical Properties
  • Resistance
  • Substrates

Fields of Study

  • Materials science

Readers

  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene