Tailoring of Grain Boundary Chemistry to Produce Super Creep-Resistant Alumina

Abstract

The influence of multi-valent dopants in diffusion related phenomena is complex. For situations where grain boundary diffusion predominates, factors such as grain boundary segregation and compensating defects may have countervailing influences. These are highly pertinent issues when considering the efficacy of high temperature coatings, where failure of the underlying substrate is driven by oxidation. Accordingly, the influence of impurities on the rates of both inward diffusion of oxygen, and outward cation diffusion is critical. On this note, work has initiated on simulating the distribution of a diffusing species within a medium where both rapid and slow diffusion paths exist. In practice this could be a sintered polycrystal, a thermally sprayed coating, or a fibrous composite material. Once developed, it is believed that such a model would be a valuable tool in the lifetime prediction of components, as well as the design and selection of oxidation resistant coatings.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 2003
Accession Number
ADA420738

Entities

People

  • Helen M. Chang
  • Jeffrey M. Rickman
  • Martin P Harmer

Organizations

  • Lehigh University

Tags

Communities of Interest

  • Human Systems

DTIC Thesaurus Topics

  • Advanced Materials
  • Boundaries
  • Chemistry
  • Coatings
  • Composite Materials
  • Creep
  • Diffusion
  • Grain Boundaries
  • Grain Growth
  • Grain Size
  • High Temperature
  • Impurities
  • Materials
  • Materials Science
  • Oxidation
  • Partial Pressure
  • Polycrystals

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Powder metallurgy of Titanium alloys.
  • Surface Engineering/Surface Coating Technology.