Nanotube/Polymer Composites: Materials Selection and Process Design

Abstract

The objectives of this project were (1) establish proof of principle by demonstrating enhanced polymer properties by the addition of single walled nanotubes (SWNTs), (2) provide guidelines for materials selection that give improved mechanical, electrical and/or thermal properties, and (3) define processing methods most appropriate for the materials identified. Our study of SWNT-polymer composites focuses on thermoplastics, because these materials can be readily drawn into fibers. As we have shown previously, the extensional flow exerted on the composite during fiber spinning aligns the SWNT to an unprecedented level. The anisotropic orientation of SWNT in these composite fibers provides an advantage when bolting for changes in macroscopic properties, particularly tensile strength. Composite processing and composite characterization received comparable effort in this project. Processing efforts include our coagulation method as well as in situ polymerization of nylon in the presence of well-dispersed SWNT. In addition to mechanical testing of the SWNT-thermoplastic fibers, we established methods for testing the electrical and thermal conductivity of these highly anisotropic materials. We used scattering methods for quantifying the extent of dispersion within the composites, a widely appreciated and long standing question in nanocomposites.

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Document Details

Document Type
Technical Report
Publication Date
May 19, 2004
Accession Number
ADA423465

Entities

People

  • John E. Fischer
  • Karen I Winey

Organizations

  • University of Pennsylvania

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Carbon Nanotubes
  • Composite Materials
  • Conductivity
  • Fiber Spinning
  • Fibers
  • Fullerenes
  • Materials
  • Materials Processing
  • Mechanical Properties
  • Nanocomposites
  • Polymer Matrix Composites
  • Polymers
  • Scattering
  • Tensile Strength
  • Thermal Conductivity
  • Thermal Properties
  • Thermoplastic Resins

Fields of Study

  • Materials science

Readers

  • Nanocomposite Materials Science
  • Reinforced Composite Materials