Infrared Stark Effect Spectroscopy for Interface Characterization

Abstract

The aim of this project is to develop a technique that can be used to obtain information concerning the formation of chemical bonds, which relate to adhesion strength, at interfaces. The technique being developed is based on the application of a large electric field in the interface region of a multiplayer structure, and then using the field to Stark shift the infrared signals from the chemical bonds between the layers. Much of the work conducted over this report period was focused on improving the signal-to-noise ratio performance of the Stark shift infrared spectrometer. Significant noise sources were identified and a new interleaved operational mode of the spectrometer implemented that avoids the largest of the noise components. We also discuss the use of an epitaxially grown layer of silicon as an adhesion layer for structures consisting of a silica sol-gel film on a crystalline germanium substrate. The very thin silicon layer does not measurably affect the optical properties of these composite systems and solves the delamination problem that has limited the utility of these structures. We are now focusing on the application of the new infrared technique to polymer/metal systems and to the study of self-assembled monolayer systems with unique properties such as temperature driven phase transitions.

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Document Details

Document Type
Technical Report
Publication Date
Nov 11, 2002
Accession Number
ADA428899

Entities

People

  • Thomas M. Niemczyk

Organizations

  • University of New Mexico

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Adhesion
  • Chemical Bonds
  • Chemistry
  • Composite Materials
  • Films
  • Infrared Spectrometers
  • Materials
  • Monomolecular Films
  • Optical Properties
  • Phase Transformations
  • Spectra
  • Spectrometers
  • Spectroscopy
  • Stark Effect
  • Surface Plasmon Resonance
  • Surface Plasmons
  • Surface Properties

Readers

  • Nanocomposite Materials Science
  • Semiconductor Device Technology
  • Systems Analysis and Design