Quantiative and Qualitative Determination of Organics in Water Using Electrospray Ionization Coupled With Ion Mobility Spectrometry

Abstract

The primary objectives of this research were to determine the capabilities of ESI-IMS for monitoring of aqueous samples containing chemical warfare agents or their subsequent degradation products. Rapid analysis times, excellent sensitivity, and potential portability make IMS an excellent tool for field applications. The ion chemistry for several chemical warfare degradation products were studied both with a prototype instrument and a high-resolution ESI-IMS instrument coupled with a quadrupole mass spectrometer (MS), showing excellent sensitivities for these compounds. Also, the ability to directly monitor water samples without prior sample preparation was shown. A portable ESI-IMS instrument has been designed and constructed. A high resolution ESI-IMS instrument coupled with a time of flight MS was assembled and showed excellent sensitivities for several chemical warfare degradation compounds. Due to the time compatibility of IMS and TOFMS, nine compounds were all resolved in two dimensions (mobility and m/z) within a minute.

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Document Details

Document Type
Technical Report
Publication Date
Apr 28, 2003
Accession Number
ADA429060

Entities

People

  • Herbert H. Hill Jr.

Organizations

  • Washington State University

Tags

Communities of Interest

  • Human Systems

DTIC Thesaurus Topics

  • Analytical Chemistry
  • Chemical Analysis
  • Chemical Warfare
  • Chemical Warfare Agents
  • Chemistry
  • Electrospray
  • Electrospray Ionization
  • High Resolution
  • Instrumentation
  • Ionization
  • Mass Spectra
  • Mass Spectrometers
  • Mass Spectrometry
  • Mobility
  • Spectrometers
  • Spectrometry
  • Warfare

Readers

  • Analytical Chemistry