Synthesis, Characterization, and Structural Investigations of 1-amino-3-Substituted-1,2,3-Triazolium Salts, and a New Route to 1-substituted-1,2,3-triazoles

Abstract

Quarternary salts based upon 3-alkyl substituted 1-amino-1,2,3-triazolium cations (alkyl = methyl, ethyl, n-propyl, 2-propenyl, and n-butyl) have been synthesized and characterized by vibrational spectra, multinuclear NMR, elemental analysis, and DSC studies. Subsequent diazotization of these salts results in the exclusive formation of 1-alkyl-1,2,3-triazoles. Single crystal x-ray studies were carried out for 1-amino-3- methyl-1,2,3-triazolium iodide, 1-amino-3-ethyl-1,2,3-triazolium bromide, 1-amino-3-npropyl- 1,2,3-triazolium bromide, and 1-amino-3-n-butyl-1,2,3-triazolium bromide as well as the starting heterocycle, 1-amino-1,2,3-triazole, and all of the structures are discussed.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2004
Accession Number
ADA433942

Entities

People

  • Gregory Kaplan
  • Gregory W. Drake
  • Kerri Tollison
  • Leslie Hall
  • Tommy Hawkins

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Air Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Air Force Research Laboratories
  • Alcohols
  • Chemical Synthesis
  • Chemistry
  • Crystal Structure
  • Crystallography
  • Crystals
  • Diffraction
  • Mass Spectrometry
  • Materials
  • Physical Properties
  • Single Crystals
  • Spectra
  • Spectroscopy
  • Vibrational Spectra
  • X Rays
  • X-Ray Crystallography

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry