Exploiting Novel Calcium-Mediated Apoptotic Processes for the Treatment of Human Breast

Abstract

Alterations in the regulation and initiation of cell death, in particular caspase-mediated apoptotic cell death, have been associated with a vast array of pathological disease states such as cancer, and the development of resistance to cancer chemotherapies. Beta-Lapachone (Beta-Lap), a naturally occurring 1,2 naphthoquinone, has been shown by our laboratory to induce non-caspase-mediated apoptosis in breast and prostate cancer cells that express the two electron oxidoreductase, NAD(P)H:quinone oxidoreductase(NQO1). Here, we demonstrate that poly(ADP)-ribose polymerase (PARP) hyperactivation, occurs shortly after Beta-lap exposure in an NQO1 dependent manner. Hyperactivation of PARP is consistent with the presence of DNA strand breaks detected by comet and gammaH2AX formation. Chemical Inhibition of PARP activity in MCF-7 human breast cancer cells by 3-aminobenzamide or DPQ suppressed beta-lab-induced apoptosis consistent with a role for PARP hyperactivation in beta-lap induced cell death. Chelation of Interacellular Ca2+ using BATPA-AM after beta-lap treatment abrogated gammaH2AX formation, PARP activation, and dramatically blocked beta-lap induced death as measured by long-term growth assays. Collectively, these data demonstrate the importance of Ca2+ mediated PARP hyperactivation in beta-lab-induced cell death. We will discuss how this Ca2+ dependent cell death can be exploited to effectively target and treat tumors that have lost their ability to undergo caspase-mediated apoptosis.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 2005
Accession Number
ADA434112

Entities

People

  • David A. Boothman
  • Melissa S. Bentle

Organizations

  • Case Western Reserve University

Tags

DTIC Thesaurus Topics

  • Amino Acids
  • Apoptosis
  • Breast Cancer
  • Cell Line
  • Cell Physiological Processes
  • Cells
  • Chemistry
  • Chemotherapy
  • Epithelial Cells
  • Inhibition
  • Kinases
  • Neoplasms
  • Programmed Cell Death
  • Prostate Cancer
  • Proteins
  • Quinones
  • Tumor Cell Line

Fields of Study

  • Biology

Readers

  • Cellular and Molecular Pathways of Apoptosis.
  • Molecular and Cellular Biochemistry
  • Oncology

Technology Areas

  • Microelectronics